Наблюдение и природа химических волн в реакциях окислительного катализа на платиновых металлах
Диссертация
Проведенные исследования вносят существенный вклад в изучение закономерностей протекания автоколебаний и химических волн в реакциях окислительного катализа, что позволяет наиболее близко подойти к изучению катализа на атомарном уровне, необходимому для понимания механизма действия реальных нанесенных высокодисперсных металлических катализаторов, в которых ограненные кристаллиты металлов… Читать ещё >
Содержание
- Глава 1. ЛИТЕРАТУРНЫЙ ОБЗОР И 1Л, Механизмы окислительного катализа модельных реакций на платиновых металлах с участием молекулярных и диссоциативных форм адсорбции реактантов: Ог СО, Н2, N
- 1. Л. 1. Современные подходы в изучении окислительного катализа на металлах
- 1. 1. 2. Адсорбция СО и 02 на платиновых металлах
- 1. 1. 3. Окисление окиси углерода. Образование «возбуждённых» молекул С
- 1. 1. 4. Окисление водорода
- 1. 2. Природа автоколебаний и химических волн на монокристаллах металлов
- 1. 2. 1. Механизм с «фазовым» переходом и с «реконструкцией»
- 1. 2. 2. Окислительно — восстановительный или «оксидный» механизм
- 1. 2. 3. «Углеродная» модель автоколебаний
- 1. 2. 4. «Вакантная» модель автоколебаний
- 1. 2. 5. «Термокинетические» автоколебания и «тепловые» волны
- 1. 3. Математические модели описания автоколебаний и химических волн
- 1. Л. 1. Современные подходы в изучении окислительного катализа на металлах
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